Selecting the best or most appropriate finding aid for identifying sources depends almost entirely on the context of your research assignment. There is no single database or web search interface that will work for every research context; instead, you'll need to match your specific research needs to a variety of options.
Library catalog searches (i.e., Primo) can be the better choice when you are seeking in-depth, book-length treatments of a topic, or want to find an encyclopedia or other tertiary source.
Multidisciplinary databases (i.e., JSTOR) can be the most appropriate choice when you just want to get a sense of what's available on a topic and when it isn't so important that you pay attention to disciplinary lenses.
Subject databases (i.e., Philosopher's Index) are the best choice for identifying the widest range of sources on a topic within a specific academic discipline. Recommended subject databases for each discipline can be found on the "articles" tab in each library subject guide.